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Journal Articles

Magnetic and orbital fluctuations in filled skutterudites

Hotta, Takashi

Physica B; Condensed Matter, 378-380, p.51 - 53, 2006/05

 Times Cited Count:4 Percentile:22.72(Physics, Condensed Matter)

In order to clarify what types of spin and orbital fluctuations dominate over low-temperature electronic properties of Pr-based filled skutterudites, we evaluate multipole susceptibility based on a multiorbital Anderson model constructed from a $$j$$-$$j$$ coupling scheme. It is found that magnetic and quadrupole fluctuations are dominant at low temperatures. When we further include the effect of rattling as dynamical Jahn-Teller phonons, there remain quadrupole and octupole fluctuations, which may induce exotic superconducting pairing.

Journal Articles

Multipole fluctuations in filled skutterudites

Hotta, Takashi

Journal of the Physical Society of Japan, 74(9), p.2425 - 2429, 2005/09

 Times Cited Count:26 Percentile:73.56(Physics, Multidisciplinary)

In order to clarify exotic multipole properties of filled skutterudites, we evaluate multipole susceptibility for $$n$$=1$$sim$$5, where $$n$$ is the local $$f$$-electron number, on the basis of a multiorbital Anderson model constructed using the $$j$$-$$j$$ coupling scheme. For $$n$$=1, magnetic fluctuations dominate over low-temperature electronic properties, while for $$n$$=2 and 4, electronic states are dominated by both magnetic and quadrupole fluctuations. For $$n$$=3 and 5, octupole fluctuations are found to be significant, depending on the crystalline electric field potential. We discuss possible relevance of the results to actual materials.

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